Using a pastry brush, brush lemon simple syrup onto each of the cake layers.
Place a cake layer face-up on cake plate or 10″ round thin cake board.
Place about 1 cup of frosting on top, and spread evenly with a small offset palette knife.
Repeat step 1-2 until one layer remains.
Place final layer, face-down (bottom of cake layer is facing up). Place a generous scoop of frosting on top, spreading evenly with an offset palette knife and working your way down the sides until you have a very thin layer of frosting over the entire cake and any holes have been filled. Use a bench scraper to achieve very smooth sides. Chill until set — about 30 minutes.
Remove from refrigerator and cover with a final, thicker layer of frosting.
Finish with any decorations of choice, or frosting borders. I added a bit more powdered sugar to the remaining frosting to stiffen it up a bit and did a simple piped border around the top and bottom edges of the cake, and topped with decorated skewers (Search Pinterest for cute decorating ideas!).
Store in a cake keeper at room temperature for up to 2 days, or in refrigerator for up to 5 days. As with most cakes, it’s best eaten the day it's made.